徐艺 研究员 徐艺 研究员

最小化 最大化

徐艺 研究员

联系方式：yixusheldon@iccas.ac.cn

个人简介

徐艺，中国科学院化学研究所研究员，博士生导师。分别于2016年、2021年在加拿大多伦多大学获得学士与博士学位；2022年进入美国斯坦福大学从事博士后研究工作，2024年作为国家高层次引进人才全职加入中国科学院化学研究所。从事电化学反应器设计与微纳尺度传质理论研究，交叉结合精细化工、流体数值模拟和人工智能等相关技术方向，研发面向碳中和与新能源的异相电化学反应系统。近年来在相关领域累计发表第一或通讯作者文章10篇，包括Joule. (3篇)、Energy Environ. Sci. (2篇)、Nat. Commun. (2篇)、Angew. Chem. Int. Ed.、ACS Energy Lett.等。获得加拿大班廷学者基金（每年授予70人）、以项目导师身份带领团队获2021届埃隆·马斯克XPrize for Carbone Removal CO2技术竞赛奖(全球23支团队)、中国国家优秀自费留学生奖学金（每年授予500人）、加拿大博士研究生国家奖学金等重要奖项。

 

研究方向

二氧化碳电化学还原

二氧化碳电化学大气碳捕捉

氮气电化学还原

 

教育背景

2012.9-2016.7 加拿大多伦多大学，本科

2016.9-2021.1 加拿大多伦多大学，博士

 

工作经历

2021.1-2022.3 加拿大多伦多大学，博士后研究员

2022.3-2024.3 美国斯坦福大学，博士后研究员

2024.3-2024.5 中国科学院化学研究所，高级访问学者

2024.5-今 中国科学院化学研究所，中国科学院胶体、界面与化学热力学重点实验室，研究员

 

论文发表

  1. Xu, Y., Liu, S., Edwards, J. P., Huang, J. E., Sargent, E. H. & Sinton, D. Regeneration of direct air CO2 capture liquid via alternating electrocatalysis. Joule 7,7 2107-2117 (2023).
  2. Xu, Y., Miao, R. K., Edwards, J. P., Robb, A., Liu, S., O’Brien, C. P., Gabardo, C. M., Fan, M., Huang, J. E., Sargent, E. H. & Sinton, D. A Microchanneled Solid Electrolyte for Carbon-Efficient CO2 Electrolysis. Joule 6, 6 1333-1343. (2022).
  3. Xu, Y., Li, F., Xu, A., Edwards, J. P., Hung, S., Gabardo, C. M., O’Brien, Liu, S., Wang, X., Li, Y., Wicks, J., Miao, R., Liu, Y., Li, J., Huang, J., Abed, J., Wang, Y., Sargent, E. H. & Sinton, D. Low coordination number copper catalysts for electrochemical CO2 methanation in a membrane electrode assembly. Nat. Commun., 12, 29324 (2021).
  4.  Xu, Y., Edwards, J. P., Liu, S., Miao, R. K., Huang, J. E., Gabardo, C. M., O’Brien, C. P., Li, J., Sargent, E. H. & Sinton, D. Self-Cleaning CO2 Reduction Systems: Unsteady Electrochemical Forcing Enables Stability. ACS Energy Lett. 6, 809–815 (2021).
  5. Xu, Y., Edwards, J. P., Zhong, J., O’Brien, C. P., Gabardo, C. M., McCallum, C., Li, J., Dinh, C.-T., Sargent, E. H. & Sinton, D. Oxygen-tolerant electroproduction of C2 products from simulated flue gas. Energy Environ. Sci. 13, 554–561 (2020).
  6. Xu, Y., Riordon, J., Cheng, X., Bao, B. & Sinton, D. The Full Pressure–Temperature Phase Envelope of a Mixture in 1000 Microfluidic Chambers. Angew. Chemie - Int. Ed. 56, 13962–13967 (2017).
  7. Liu, S., Zhang, J.,Li, F.,Edwards, J.P.,Xiao, Y. C.,Kim, D.,Papangelakis, P.,Kim, J.,Elder, D.,De Luna, P.,Fan, M.,Lee, G.,Miao, R.K.,Ghosh, T.,Yan, Y.,Chen, Y.,Zhao, Y.,Guo, Z.,Tian, C.,Li, P.,Xu, Y.*, Sargent, E. H.*&  Sinton, D.* , Direct air capture of CO2 via cyclic viologen electrocatalysis.Energy Environ. Sci.17, 1266-1278 (2024).
  8.  Fan, M.*, Miao, R. K.*, Ou, P.*, Xu, Y.*, Lin, Z.-Y., Lee, T.-J., Hung, S.-F., Xie, K., Huang, J. E., Ni, W., Li, J., Zhao, Y., Ozden, A., O’Brien, C. P., Chen, Y., Xiao, Y. C., Liu, S., Wicks, J., Wang, X., et al. Single-site decorated copper enables energy- and carbon-efficient CO2 methanation in acidic conditions. Nat Commun 14, 3314 (2023).
  9. Miao, R. K.*, Xu, Y.*, Ozden, A., Robb, A., O’Brien, C. P., Gabardo, C. M., Lee, G., Edwards, J. P., Huang, J. E., Fan, M., Wang, X., Liu, S., Yan, Y., Sargent, E. H. & Sinton, D. Electroosmotic flow steers neutral products and enables concentrated ethanol electroproduction from CO2. Joule 5, 10, 2742-2753. (2021)
  10. Edwards, J. P.*, Xu, Y.*, Gabardo, C. M., Dinh, C.-T., Li, J., Qi, Z., Ozden, A., Sargent, E. H. & Sinton, D. Efficient electrocatalytic conversion of carbon dioxide in a low-resistance pressurized alkaline electrolyzer. Appl. Energy 261, 114305 (2020).                                                                                                                               
    其余已发表合著论文
  11. Chen, Y., Li, X.-Y., Chen, Z., Ozden, A., Huang, J. E., Ou, P., Dong, J., Zhang, J., Tian, C., Lee, B.-H., Wang, X., Liu, S., Qu, Q., Wang, S., Xu, Y., Miao, R. K., Zhao, Y., Liu, Y., Qiu, C., et al. Efficient multicarbon formation in acidic CO2 reduction via tandem electrocatalysis. Nat Nanotechnol (2023) doi:10.1038/s41565-023-01543-8.
  12. Lee, D. U., Joensen, B., Jenny, J., Ehlinger, V. M., Lee, S.-W., Abiose, K., Xu, Y., Sarkar, A., Lin, T. Y., Hahn, C. & Jaramillo, T. F. Controlling Mass Transport in Direct Carbon Dioxide Zero-Gap Electrolyzers via Cell Compression. ACS Sustain Chem Eng 11, 16661–16668 (2023).
  13. Miao, R. K., Wang, N., Hung, S.-F., Huang, W.-Y., Zhang, J., Zhao, Y., Ou, P., Wang, S., Edwards, J. P., Tian, C., Han, J., Xu, Y., Fan, M., Huang, J. E., Xiao, Y. C., Ip, A. H., Liang, H., Sargent, E. H. & Sinton, D. Electrified Cement Production via Anion-Mediated Electrochemical Calcium Extraction. ACS Energy Lett 8, 4694–4701 (2023).
  14. Fan, M., Huang, J. E., Miao, R. K., Mao, Y., Ou, P., Li, F., Li, X.-Y., Cao, Y., Zhang, Z., Zhang, J., Yan, Y., Ozden, A., Ni, W., Wang, Y., Zhao, Y., Chen, Z., Khatir, B., O’Brien, C. P., Xu, Y., et al. Cationic-group-functionalized electrocatalysts enable stable acidic CO2 electrolysis. Nat Catal 6, 763–772 (2023).
  15. Jin, J., Wicks, J., Min, Q., Li, J., Hu, Y., Ma, J., Wang, Y., Jiang, Z., Xu, Y., Lu, R., Si, G., Papangelakis, P., Shakouri, M., Xiao, Q., Ou, P., Wang, X., Chen, Z., Zhang, W., Yu, K., et al. Constrained C2 adsorbate orientation enables CO-to-acetate electroreduction. Nature 617, 724–729 (2023).
  16. Niemann, V. A., Benedek, P., Guo, J., Xu, Y., Blair, S. J., Corson, E. R., Nielander, A. C., Jaramillo, T. F. & Tarpeh, W. A. Co-designing Electrocatalytic Systems with Separations To Improve the Sustainability of Reactive Nitrogen Management. ACS Catal 13, 6268–6279 (2023).
  17. Luo, M., Ozden, A., Wang, Z., Li, F., Erick Huang, J., Hung, S., Wang, Y., Li, J., Nam, D., Li, Y. C., Xu, Y., Lu, R., Zhang, S., Lum, Y., Ren, Y., Fan, L., Wang, F., Li, H., Appadoo, D., et al. Coordination Polymer Electrocatalysts Enable Efficient CO‐to‐Acetate Conversion. Advanced Materials 35, 2209567 (2023).
  18. Zhao, Y., Hao, L., Ozden, A., Liu, S., Miao, R. K., Ou, P., Alkayyali, T., Zhang, S., Ning, J., Liang, Y., Xu, Y., Fan, M., Chen, Y., Huang, J. E., Xie, K., Zhang, J., O’Brien, C. P., Li, F., Sargent, E. H., et al. Conversion of CO2 to multicarbon products in strong acid by controlling the catalyst microenvironment. Nature Synthesis 2, 403–412 (2023).
  19. Xiao, Y. C., Gabardo, C. M., Liu, S., Lee, G., Zhao, Y., O’Brien, C. P., Miao, R. K., Xu, Y., Edwards, J. P., Fan, M., Huang, J. E., Li, J., Papangelakis, P., Alkayyali, T., Sedighian Rasouli, A., Zhang, J., Sargent, E. H. & Sinton, D. Direct carbonate electrolysis into pure syngas. EES Catalysis 1, 54–61 (2023).
  20. Li, Y., Ozden, A., Leow, W. R., Ou, P., Huang, J. E., Wang, Y., Bertens, K., Xu, Y., Liu, Y., Roy, C., Jiang, H., Sinton, D., Li, C. & Sargent, E. H. Redox-mediated electrosynthesis of ethylene oxide from CO2 and water. Nat Catal 5, 185–192 (2022).
  21. Robb, A., Ozden, A., Miao, R. K., O’Brien, C. P., Xu, Y., Gabardo, C. M., Wang, X., Zhao, N., García de Arquer, F. P., Sargent, E. H. & Sinton, D. Concentrated Ethanol Electrosynthesis from CO2 via a Porous Hydrophobic Adlayer. ACS Appl Mater Interfaces 14, 4155–4162 (2022).
  22. McCallum, C., Gabardo, C. M., O’Brien, C. P., Edwards, J. P., Wicks, J., Xu, Y., Sargent, E. H. & Sinton, D. Reducing the crossover of carbonate and liquid products during carbon dioxide electroreduction. Cell Rep Phys Sci 2, 100522 (2021).
  23. O’Brien, C. P., Miao, R. K., Liu, S., Xu, Y., Lee, G., Robb, A., Huang, J. E., Xie, K., Bertens, K., Gabardo, C. M., Edwards, J. P., Dinh, C.-T., Sargent, E. H. & Sinton, D. Single Pass CO2 Conversion Exceeding 85% in the Electrosynthesis of Multicarbon Products via Local CO2 Regeneration. ACS Energy Lett 6, 2952–2959 (2021).
  24. Huang, J. E., Li, F., Ozden, A., Sedighian Rasouli, A., García de Arquer, F. P., Liu, S., Zhang, S., Luo, M., Wang, X., Lum, Y., Xu, Y., Bertens, K., Miao, R. K., Dinh, C.-T., Sinton, D. & Sargent, E. H. CO2 electrolysis to multicarbon products in strong acid. Science (1979) 372, 1074–1078 (2021).
  25. Wang, X., Ou, P., Wicks, J., Xie, Y., Wang, Y., Li, J., Tam, J., Ren, D., Howe, J. Y., Wang, Z., Ozden, A., Finfrock, Y. Z., Xu, Y., Li, Y., Rasouli, A. S., Bertens, K., Ip, A. H., Graetzel, M., Sinton, D., et al. Gold-in-copper at low *CO coverage enables efficient electromethanation of CO2. Nat Commun 12, 3387 (2021).
  26. Li, J., Ozden, A., Wan, M., Hu, Y., Li, F., Wang, Y., Zamani, R. R., Ren, D., Wang, Z., Xu, Y., Nam, D., Wicks, J., Chen, B., Wang, X., Luo, M., Graetzel, M., Che, F., Sargent, E. H. & Sinton, D. Silica-copper catalyst interfaces enable carbon-carbon coupling towards ethylene electrosynthesis. Nat Commun 12, 2808 (2021).
  27. Li, Y., Xu, A., Lum, Y., Wang, X., Hung, S.-F., Chen, B., Wang, Z., Xu, Y., Li, F., Abed, J., Huang, J. E., Rasouli, A. S., Wicks, J., Sagar, L. K., Peng, T., Ip, A. H., Sinton, D., Jiang, H., Li, C., et al. Promoting CO2 methanation via ligand-stabilized metal oxide clusters as hydrogen-donating motifs. Nat Commun 11, 6190 (2020).
  28. Li, J., Xu, A., Li, F., Wang, Z., Zou, C., Gabardo, C. M., Wang, Y., Ozden, A., Xu, Y., Nam, D.-H., Lum, Y., Wicks, J., Chen, B., Wang, Z., Chen, J., Wen, Y., Zhuang, T., Luo, M., Du, X., et al. Enhanced multi-carbon alcohol electroproduction from CO via modulated hydrogen adsorption. Nat Commun 11, 3685 (2020).
  29. Wang, Y., Wang, Z., Dinh, C.-T., Li, J., Ozden, A., Kibria, M. G., Seifitokaldani, A., Tan, C.-S., Gabardo, C. M. Luo, M. & Xu, Y. Catalyst synthesis under CO2 electroreduction favours faceting and promotes renewable fuels electrosynthesis. Nat Catal 3, 98–106 (2020).
  30. Wang, X., Xu, A., Li, F., Hung, S.-F., Nam, D.-H., Gabardo, C. M., Wang, Z., Xu, Y., Ozden, A., Rasouli, A. S., Ip, A. H., Sinton, D. & Sargent, E. H. Efficient Methane Electrosynthesis Enabled by Tuning Local CO2 Availability. J Am Chem Soc 142, 3525–3531 (2020).
  31. Zhong, J., Alibakhshi, M. A., Xie, Q., Riordon, J., Xu, Y., Duan, C. & Sinton, D. Exploring Anomalous Fluid Behavior at the Nanoscale: Direct Visualization and Quantification via Nanofluidic Devices. Acc Chem Res 53, 347–357 (2020).
  32. Li, F., Li, Y. C., Wang, Z., Li, J., Nam, D. H., Lum, Y., Luo, M., Wang, X., Ozden, A., Hung, S. F., Chen, B., Wang, Y., Wicks, J., Xu, Y., Li, Y., Gabardo, C. M., Dinh, C. T., Wang, Y., Zhuang, T. T., et al. Cooperative CO2-to-ethanol conversion via enriched intermediates at molecule–metal catalyst interfaces. Nat Catal 3, 75–82 (2020).
  33. Li, F., Thevenon, A., Rosas-Hernández, A., Wang, Z., Li, Y., Gabardo, C. M., Ozden, A., Dinh, C. T., Li, J., Wang, Y., Edwards, J. P., Xu, Y., McCallum, C., Tao, L., Liang, Z.-Q., Luo, M., Wang, X., Li, H., O’Brien, C. P., et al. Molecular tuning of CO2-to-ethylene conversion. Nature 577, 509–513 (2020).
  34. Li, J., Wang, Z., McCallum, C., Xu, Y., Li, F., Wang, Y., Gabardo, C. M., Dinh, C.-T., Zhuang, T.-T. & Wang, L. Constraining CO coverage on copper promotes high-efficiency ethylene electroproduction. Nat Catal 2, 1124–1131 (2019).
  35. Gabardo, C. M., O’Brien, C. P., Edwards, J. P., McCallum, C., Xu, Y., Dinh, C.-T., Li, J., Sargent, E. H. & Sinton, D. Continuous Carbon Dioxide Electroreduction to Concentrated Multi-carbon Products Using a Membrane Electrode Assembly. Joule 3, 2777–2791 (2019).
  36. Wang, Y., Riordon, J., Kong, T., Xu, Y., Nguyen, B., Zhong, J., You, J. B., Lagunov, A., Hannam, T. G., Jarvi, K. & Sinton, D. Prediction of DNA Integrity from Morphological Parameters Using a Single‐Sperm DNA Fragmentation Index Assay. Advanced Science 6, 1900712 (2019).
  37. Pang, Y., Li, J., Wang, Z., Tan, C.-S., Hsieh, P.-L., Zhuang, T.-T., Liang, Z.-Q., Zou, C., Wang, X., de Luna, P., Edwards, J. P., Xu, Y., Li, F., Dinh, C.-T., Zhong, M., Lou, Y., Wu, D., Chen, L.-J., Sargent, E. H., et al. Efficient electrocatalytic conversion of carbon monoxide to propanol using fragmented copper. Nat Catal 2, 251–258 (2019).
  38. Zhao, Y., Wang, Y., Zhong, J., Xu, Y., Sinton, D. & Jin, Z. Bubble point pressures of hydrocarbon mixtures in multiscale volumes from density functional theory. Langmuir 34, 14058–14068 (2018).
  39. Zhong, J., Zhao, Y., Lu, C., Xu, Y., Jin, Z., Mostowfi, F. & Sinton, D. Nanoscale phase measurement for the shale challenge: multicomponent fluids in multiscale volumes. Langmuir 34, 9927–9935 (2018).
  40. Jatukaran, A., Zhong, J., Persad, A. H., Xu, Y., Mostowfi, F. & Sinton, D. Direct Visualization of Evaporation in a Two-Dimensional Nanoporous Model for Unconventional Natural Gas. ACS Appl Nano Mater 1, 1332–1338 (2018).
  41. Zhong, J., Riordon, J., Zandavi, S. H., Xu, Y., Persad, A. H., Mostowfi, F. & Sinton, D. Capillary condensation in 8 nm deep channels. J Phys Chem Lett 9, 497–503 (2018).
  42. Zhong, J., Abedini, A., Xu, L., Xu, Y., Qi, Z., Mostowfi, F. & Sinton, D. Nanomodel visualization of fluid injections in tight formations. Nanoscale 10, 21994–22002 (2018).
  43. Qi, Z., Xu, L., Xu, Y., Zhong, J., Abedini, A., Cheng, X. & Sinton, D. Disposable silicon-glass microfluidic devices: precise, robust and cheap. Lab Chip 18, 3872–3880 (2018).
  44. Zhong, J., Talebi, S., Xu, Y., Pang, Y., Mostowfi, F. & Sinton, D. Fluorescence in sub-10 nm channels with an optical enhancement layer. Lab Chip (2018) doi:10.1039/C7LC01193H.
  45. Li, H., Zhong, J., Pang, Y., Zandavi, S. H., Persad, A. H., Xu, Y., Mostowfi, F. & Sinton, D. Direct visualization of fluid dynamics in sub-10 nm nanochannels. Nanoscale 9, 9556–9561 (2017).
  46. Bao, B., Riordon, J., Xu, Y., Li, H. & Sinton, D. Direct Measurement of the Fluid Phase Diagram. Anal Chem 88, 6986–6989 (2016).